Publications from 2021

27. A perspective on scaling up quantum computation with molecular spins

S. Carretta, D. Zueco, A. Chiesa, Á. Gómez-León, F. Luis
Artificial magnetic molecules can contribute to progressing toward large scale quantum computation by (a) integrating multiple quantum resources and (b) reducing the computational costs of some applications. Chemical design, guided by theoretical proposals, allows embedding nontrivial quantum functionalities in each molecular unit, which then acts as a microscopic quantum processor able to encode error protected logical qubits or to implement quantum simulations. Scaling up even further requires “wiring-up” multiple molecules. We discuss how to achieve this goal by the coupling to on-chip superconducting resonators. The potential advantages of this hybrid approach and the challenges that still lay ahead are critically reviewed.

26. Automatic design of quantum feature maps

Sergio Altares-López, Angela Ribeiro, Juan José García-Ripoll
We propose a new technique for the automatic generation of optimal ad-hoc ans\”atze for classification by using quantum support vector machine (QSVM). This efficient method is based on NSGA-II multiobjective genetic algorithms which allow both maximize the accuracy and minimize the ansatz size. It is demonstrated the validity of the technique by a practical example with a non-linear dataset, interpreting the resulting circuit and its outputs. We also show other application fields of the technique that reinforce the validity of the method, and a comparison with classical classifiers in order to understand the advantages of using quantum machine learning.

25. Cold atoms meet lattice gauge theory

Monika Aidelsburger, Luca Barbiero, Alejandro Bermudez, Titas Chanda, Alexandre Dauphin, Daniel González-Cuadra, Przemysław R. Grzybowski, Simon Hands, Fred Jendrzejewski, Johannes Jünemann, Gediminas Juzeliūnas, Valentin Kasper, Angelo Piga, Shi-Ju Ran, Matteo Rizzi, Germán Sierra, Luca Tagliacozzo, Emanuele Tirrito, Torsten V. Zache, Jakub Zakrzewski, Erez Zohar, Maciej Lewenstein
The central idea of this review is to consider quantum field theory models relevant for particle physics and replace the fermionic matter in these models by a bosonic one. This is mostly motivated by the fact that bosons are more ‘accessible’ and easier to manipulate for experimentalists, but this ‘substitution’ also leads to new physics and novel phenomena. It allows us to gain new information about among other things confinement and the dynamics of the deconfinement transition. We will thus consider bosons in dynamical lattices corresponding to the bosonic Schwinger or Z2 Bose–Hubbard models. Another central idea of this review concerns atomic simulators of paradigmatic models of particle physics theory such as the Creutz–Hubbard ladder, or Gross–Neveu–Wilson and Wilson–Hubbard models. This article is not a general review of the rapidly growing field—it reviews activities related to quantum simulations for lattice field theories performed by the Quantum Optics Theory group at ICFO and their collaborators from 19 institutions all over the world. Finally, we will briefly describe our efforts to design experimentally friendly simulators of these and other models relevant for particle physics.

24. Design of Novel Coupling Mechanisms between Superconducting Flux Qubits

Gabriel Jaumà
We have analyzed and proposed coupling mechanisms between Three Josephson Junction Flux Qubits (3JJQ). For this, we have developed a numerical method to extract the effective Hamiltonian of a system of coupled qubits via the Schrieffer-Wolff transformation (SWT). We then give a comprehensive introduction to the 3JJQ, and study it analytically by approximating its potential with a Harmonic well. With a clear understanding of the 3JJQs, we use the SWT to gain intuition about their effective dipolar interaction with the electromagnetic field, and use that intuition to propose and study analytically and numerically the capacitive coupling of two 3JJQs via a non-tunable capacitor, and the inductive coupling of two 3JJQs via a tunable Josephson Junction (dc-SQUID), showing that we are able to reproduce non-stoquastic Hamiltonians in the strong-coupling regime.

23. Dissipative Josephson effect in coupled nanolasers

Samuel Fernández-Lorenzo, Diego Porras
Josephson effects are commonly studied in quantum systems in which dissipation or noise can be neglected or do not play a crucial role. In contrast, here we discuss a setup where dissipative interactions do amplify a photonic Josephson current, opening a doorway to dissipation-enhanced sensitivity of quantum-optical interferometry devices. In particular, we study two coupled nanolasers subjected to phase coherent drivings and coupled by a coherent photon tunneling process. We describe this system by means of a Fokker-Planck equation and show that it exhibits an interesting non-equilibrium phase diagram as a function of the coherent coupling between nanolasers. As we increase that coupling, we find a non-equilibrium phase transition between a phase-locked and a non-phase-locked steady-state, in which phase coherence is destroyed by the photon tunneling process. In the coherent, phase-locked regime, an imbalanced photon number population appears if there is a phase difference between the nanolasers, which appears in the steady-state as a result of the competition between competing local dissipative dynamics and the Josephson photo-current. The latter is amplified for large incoherent pumping rates and it is also enchanced close to the lasing phase transition. We show that the Josephson photocurrent can be used to measure optical phase differences. In the quantum limit, the accuracy of the two nanolaser interferometer grows with the square of the photon number and, thus, it can be enhanced by increasing the rate of incoherent pumping of photons into the nanolasers.

22. Dynamical decoupling methods in nanoscale NMR

C. Munuera-Javaloy, R. Puebla, J. Casanova
Nuclear magnetic resonance (NMR) schemes can be applied to micron-, and nanometer-sized samples by the aid of quantum sensors such as nitrogen vacancy (NV) color centers in diamond. These minute devices allow for magnetometry of nuclear spin ensembles with high spatial and frequency resolution at ambient conditions, thus having a clear impact in different areas such as chemistry, biology, medicine, and material sciences. In practice, NV quantum sensors are driven by microwave (MW) control fields with a twofold objective: On the one hand, MW fields bridge the energy gap between NV and nearby nuclei which enables a coherent and selective coupling among them while, on the other hand, MW fields remove environmental noise on the NV leading to enhanced interrogation time. In this work we review distinct MW radiation patterns, or dynamical decoupling techniques, for nanoscale NMR applications.

21. Engineering analog quantum chemistry Hamiltonians using cold atoms in optical lattices

Javier Argüello-Luengo, Tao Shi, Alejandro González-Tudela
Using quantum systems to efficiently solve quantum chemistry problems is one of the long-sought applications of near-future quantum technologies. In a recent work [J. Argüello-Luengo et al., Nature (London) 574, 215 (2019)], ultracold fermionic atoms have been proposed for this purpose by showing us how to simulate in an analog way the quantum chemistry Hamiltonian projected in a lattice basis set. Here, we continue exploring this path and go beyond these results in several ways. First, we numerically benchmark the working conditions of the analog simulator and find less demanding experimental setups where chemistry-like behavior in three dimensions can still be observed. We also provide a deeper understanding of the errors of the simulation appearing due to discretization and finite-size effects and provide a way to mitigate them. Finally, we benchmark the simulator characterizing the behavior of two-electron atoms (He) and molecules (

20. Frequency-resolved photon correlations in cavity optomechanics

M K Schmidt, R Esteban, G Giedke, J Aizpurua, A González-Tudela
Frequency-resolved photon correlations have proven to be a useful resource to unveil nonlinearities hidden in standard observables such as the spectrum or the standard (color-blind) photon correlations. In this manuscript, we analyze the frequency-resolved correlations of the photons being emitted from an optomechanical system where light is nonlinearly coupled to the quantized motion of a mechanical mode of a resonator, but where the quantum nonlinear response is typically hard to evidence. We present and unravel a rich landscape of frequency-resolved correlations, and discuss how the time-delayed correlations can reveal information about the dynamics of the system. We also study the dependence of correlations on relevant parameters such as the single-photon coupling strength, the filtering linewidth, or the thermal noise in the environment. This enriched understanding of the system can trigger new experiments to probe nonlinear phenomena in optomechanics, and provide insights into dynamics of generic nonlinear systems.

19. Gaussian phase sensitivity of boson-sampling-inspired strategies

Antonio A. Valido, Juan José García-Ripoll

18. Generation of photonic matrix product states with Rydberg atomic arrays

Zhi-Yuan Wei, Daniel Malz, Alejandro González-Tudela, J. Ignacio Cirac

17. Hybrid quantum–classical optimization with cardinality constraints and applications to finance

Samuel Fernández-Lorenzo, Diego Porras, Juan José García-Ripoll
Tracking a financial index boils down to replicating its trajectory of returns for a well-defined time span by investing in a weighted subset of the securities included in the benchmark. Picking the optimal combination of assets becomes a challenging NP-hard problem even for moderately large indices consisting of dozens or hundreds of assets, thereby requiring heuristic methods to find approximate solutions. Hybrid quantum-classical optimization with variational gate-based quantum circuits arises as a plausible method to improve performance of current schemes. In this work we introduce a heuristic pruning algorithm to find weighted combinations of assets subject to cardinality constraints. We further consider different strategies to respect such constraints and compare the performance of relevant quantum ans\”{a}tze and classical optimizers through numerical simulations.

16. Light-matter interactions near photonic Weyl points

Iñaki García-Elcano, Jorge Bravo-Abad, Alejandro González-Tudela
Weyl photons appear when two three-dimensional photonic bands with linear dispersion are degenerate at a single momentum point, labeled as Weyl point. These points have remarkable properties such as being robust topological monopoles of Berry curvature as well as an associated vanishing density of states. In this work, we report on a systematic theoretical study of the quantum optical consequences of such Weyl photons. First, we analyze the dynamics of a single quantum emitter coupled to a Weyl photonic bath as a function of its detuning with respect to the Weyl point and study the corrresponding emission patterns, using both perturbative and exact treatments. Our calculations show an asymmetric dynamical behavior when the emitter is detuned away from the Weyl frequency, as well as different regimes of highly collimated emission, which ultimately translate in a variety of directional collective decays. Besides, we find that the incorporation of staggered mass and hopping terms in the bath Hamiltonian both enriches the observed phenomenology and increases the tunability of the interaction. Finally, we analyze the competition between the coherent and dissipative components of the dynamics for the case of two emitters and derive the conditions under which an effective interacting spin model description is valid.

15. Non-equilibrium coupling of a quartz resonator to ions for Penning-trap fast resonant detection

Joaquín Berrocal, Steffen Lohse, Francisco Domínguez, Manuel J Gutiérrez, Francisco J Fernández, Michael Block, Juan J García-Ripoll, Daniel Rodríguez

14. Optically defined cavities in driven-dissipative photonic lattices

O. Jamadi, B. Real, K. Sawicki, C. Hainaut, A. Gonzalez-Tudela, N. Pernet, I. Sagnes, M. Morassi, A. Lemaitre, L. Le Gratiet, A. Harouri, S. Ravets, J. Bloch, A. Amo
The engineering of localised modes in photonic structures is one of the main targets of modern photonics. An efficient strategy to design these modes is to use the interplay of constructive and destructive interference in periodic photonic lattices. This mechanism is at the origin of defect modes in photonic bandgaps, bound states in the continuum and compact localised states in flat bands. Here we show that in lattices of lossy resonators, the addition of external optical drives with controlled phase enlarges the possibilities of manipulating interference effects and allows designing novel types of localised modes. Using a honeycomb lattice of coupled micropillars resonantly driven with several laser spots at energies within its photonic bands we demonstrate the localisation of light in at-will geometries down to a single site. These localised modes can be seen as fully reconfigurable optical cavities with the potentiality of enhancing nonlinear effects and of controlling light-matter interactions with single site resolution.

13. Photon-Mediated Interactions near a Dirac Photonic Crystal Slab

Erik Petrovish Navarro-Barón, Herbert Vinck-Posada, Alejandro González-Tudela
Dirac energy dispersions are responsible for the extraordinary transport properties of graphene. This motivated the quest for engineering such energy dispersions also in photonics, where they have been predicted to lead to many exciting phenomena. One paradigmatic example is the possibility of obtaining power-law, decoherence-free, photon-mediated interactions between quantum emitters when they interact with such photonic baths. This prediction, however, has been obtained either by using toy-model baths, which neglect polarization effects, or by restricting the emitter position to high-symmetry points of the unit cell in the case of realistic structures. Here, we develop a semianalytical theory of dipole radiation near photonic Dirac points in realistic structures that allows us to compute the effective photon-mediated interactions along the whole unit cell. Using this theory, we are able to find the positions that maximize the emitter interactions and their range, finding a trade-off between them. Besides, using the polarization degree of freedom, we also find positions where the nature of the collective interactions changes from being coherent to dissipative ones. Thus, our results significantly improve the knowledge of Dirac light–matter interfaces and can serve as a guidance for future experimental designs.

12. Photon-Mediated Stroboscopic Quantum Simulation of a Z2 Lattice Gauge Theory

Tsafrir Armon, Shachar Ashkenazi, Gerardo García-Moreno, Alejandro González-Tudela, Erez Zohar

11. Quantum Electrodynamics in a Topological Waveguide

Eunjong Kim, Xueyue Zhang, Vinicius S. Ferreira, Jash Banker, Joseph K. Iverson, Alp Sipahigil, Miguel Bello, Alejandro González-Tudela, Mohammad Mirhosseini, Oskar Painter

10. Quantum electrodynamics in anisotropic and tilted Dirac photonic lattices

Jaime Redondo-Yuste, María Blanco de Paz, Paloma A Huidobro, Alejandro González-Tudela
One of the most striking predictions of quantum electrodynamics is that vacuum fluctuations of the electromagnetic field can lead to spontaneous emission of atoms as well as photon-mediated interactions among them. Since these processes strongly depend on the nature of the photonic bath, a current burgeoning field is the study of their modification in the presence of photons with non-trivial energy dispersions, e.g. the ones confined in photonic crystals. A remarkable example is the case of isotropic Dirac-photons, which has been recently shown to lead to non-exponential spontaneous emission as well as dissipation-less long-range emitter interactions. In this work, we show how to further tune these processes by considering anisotropic Dirac cone dispersions, which include tilted, semi-Dirac, and the recently discovered type II and III Dirac points. In particular, we show how by changing the anisotropy of the lattice one can change both the spatial shape of the interactions as well as its coherent/incoherent nature. Finally, we theoretically analyze a possible implementation based on subwavelength atomic arrays where these energy dispersions can be engineered and interfaced with quantum emitters.

9. Quantum variational optimization: The role of entanglement and problem hardness

Pablo Díez-Valle, Diego Porras, Juan José García-Ripoll
Quantum variational optimization has been posed as an alternative to solve optimization problems faster and at a larger scale than what classical methods allow. In this paper we study systematically the role of entanglement, the structure of the variational quantum circuit, and the structure of the optimization problem, in the success and efficiency of these algorithms. For this purpose, our study focuses on the variational quantum eigensolver (VQE) algorithm, as applied to quadratic unconstrained binary optimization (QUBO) problems on random graphs with tunable density. Our numerical results indicate an advantage in adapting the distribution of entangling gates to the problem’s topology, specially for problems defined on low-dimensional graphs. Furthermore, we find evidence that applying conditional value at risk type cost functions improves the optimization, increasing the probability of overlap with the optimal solutions. However, these techniques also improve the performance of Ans\”atze based on product states (no entanglement), suggesting that a new classical optimization method based on these could outperform existing NISQ architectures in certain regimes. Finally, our study also reveals a correlation between the hardness of a problem and the Hamming distance between the ground- and first-excited state, an idea that can be used to engineer benchmarks and understand the performance bottlenecks of optimization methods.

8. Qubit-photon bound states in topological waveguides with long-range hoppings

C. Vega, M. Bello, D. Porras, A. González-Tudela
Quantum emitters interacting with photonic band-gap materials lead to the appearance of qubit-photon bound states that mediate decoherence-free, tunable emitter-emitter interactions. Recently, it has been shown that when these band gaps have a topological origin, like in the photonic Su-Schrieffer-Heeger (SSH) model, these qubit-photon bound states feature chiral shapes and certain robustness to disorder. In this paper, we consider a more general situation where the emitters interact with an extended SSH photonic model with longer-range hoppings that displays a richer phase diagram than its nearest-neighbor counterpart, e.g., phases with larger winding numbers. In particular, we first study the features of the qubit-photon bound states when the emitters couple to the bulk modes in the different phases, discern their connection with the topological invariant, and show how to further tune their shape through the use of giant atoms, i.e., nonlocal couplings. Then, we consider the coupling of emitters to the edge modes appearing in the different topological phases. Here, we show that giant-atom dynamics can distinguish between all different topological phases, in contrast to the case with local couplings. Finally, we provide a possible experimental implementation of the model based on periodic modulations of circuit QED systems. Our paper enriches the understanding of the interplay between topological photonics and quantum optics.

7. Realization of a quantum perceptron gate with trapped ions

P. Huber, J. Haber, P. Barthel, J. J. García-Ripoll, E. Torrontegui, C. Wunderlich
We report the implementation of a perceptron quantum gate in an ion-trap quantum computer. In this scheme, a perceptron’s target qubit changes its state depending on the interactions with several qubits. The target qubit displays a tunable sigmoid switching behaviour becoming a universal approximator when nested with other percetrons. The procedure consists on the adiabatic ramp-down of a dressing-field applied to the target qubit. We also use two successive perceptron quantum gates to implement a XNOR-gate, where the perceptron qubit changes its state only when the parity of two input qubits is even. The applicability can be generalized to higher-dimensional gates as well as the reconstruction of arbitrary bounded continuous functions of the perceptron observables.

6. Spreading of correlations and entanglement in the long-range transverse Ising chain

J. T. Schneider, J. Despres, S. J. Thomson, L. Tagliacozzo, L. Sanchez-Palencia

5. Three-Josephson junctions flux qubit couplings

María Hita-Pérez, Gabriel Jaumà, Manuel Pino, Juan José García-Ripoll
We analyze the coupling of two flux qubits with a general many-body projector into the low-energy subspace. Specifically, we extract the effective Hamiltonians that controls the dynamics of two qubits when they are coupled via a capacitor and/or via a Josephson junction. While the capacitor induces a static charge coupling tunable by design, the Josephson junction produces a magnetic-like interaction easily tunable by replacing the junction with a superconducting quantum interference device. Those two elements allow to engineer qubits Hamiltonians with XX, YY, and ZZ interactions, including ultrastrongly coupled ones. We present an exhaustive numerical study for two three-Josephson junctions flux qubit that can be directly used in experimental work. The method developed here, namely, the numerical tool to extract qubit effective Hamiltonians at strong coupling, can be applied to replicate our analysis for general systems of many qubits and any type of coupling.

4. Topological input-output theory for directional amplification

Tomás Ramos, Juan José García-Ripoll, Diego Porras
We present a topological approach to the input-output relations of photonic driven-dissipative systems acting as directional amplifiers. Our theory relies on a mapping from the optical non-Hermitian coupling matrix to an effective topological insulator Hamiltonian. This mapping is based on the singular value decomposition of non-Hermitian coupling matrices, the inverse matrix of which determines the linear input-output response of the system. In topologically nontrivial regimes, the input-output response of the lattice is dominated by singular vectors with zero singular values that are the equivalent of zero energy states in topological insulators, leading to directional amplification of a coherent input signal. In such topological amplification regime, our theoretical framework allows us to fully characterize the amplification properties of the quantum device such as gain, bandwidth, added noise, and noise-to-signal ratio. We exemplify our ideas in a one-dimensional nonreciprocal photonic lattice, for which we derive fully analytical predictions. We show that the directional amplification is near quantum limited with a gain growing exponentially with system size N, while the noise-to-signal ratio is suppressed as sqrt(N). This suggests interesting applications of our theory for quantum signal amplification and single-photon detection.

3. Ultraviolet Laser Pulses with Multigigahertz Repetition Rate and Multiwatt Average Power for Fast Trapped-Ion Entanglement Operations

M.I. Hussain, D. Heinrich, M. Guevara-Bertsch, E. Torrontegui, J.J. García-Ripoll, C.F. Roos, R. Blatt
The conventional approach to perform two-qubit gate operations in trapped ions relies on exciting the ions on motional sidebands with laser light, which is an inherently slow process. One way to implement a fast entangling gate protocol requires a suitable pulsed laser to increase the gate speed by orders of magnitude. However, the realization of such a fast entangling gate operation presents a big technical challenge, as such the required laser source is not available off-the-shelf. For this, we have engineered an ultrafast entangling gate source based on a frequency comb. The source generates bursts of several hundred mode-locked pulses with pulse energy $\sim$800 pJ at 5 GHz repetition rate at 393.3 nm and complies with all requirements for implementing a fast two-qubit gate operation. Using a single, chirped ultraviolet pulse, we demonstrate a rapid adiabatic passage in a Ca$^+$ ion. To verify the applicability and projected performance of the laser system for inducing entangling gates we run simulations based on our source parameters. The gate time can be faster than a trap period with an error approaching $10^{-4}$.

2. Versatile Atomic Magnetometry Assisted by Bayesian Inference

R. Puebla, Y. Ban, J.F. Haase, M.B. Plenio, M. Paternostro, J. Casanova
Quantum sensors typically translate external fields into a periodic response whose frequency is then determined by analyses performed in Fourier space. This allows for a linear inference of the parameters that characterize external signals. In practice, however, quantum sensors are able to detect fields only in a narrow range of amplitudes and frequencies. A departure from this range, as well as the presence of significant noise sources and short detection times, lead to a loss of the linear relationship between the response of the sensor and the target field, thus limiting the working regime of the sensor. Here we address these challenges by means of a Bayesian inference approach that is tolerant to strong deviations from desired periodic responses of the sensor and is able to provide reliable estimates even with a very limited number of measurements. We demonstrate our method for an 171Yb+ trapped-ion quantum sensor but stress the general applicability of this approach to different systems.

1. Work statistics and symmetry breaking in an excited-state quantum phase transition

Zakaria Mzaouali, Ricardo Puebla, John Goold, Morad El Baz, Steve Campbell
We examine how the presence of an excited state quantum phase transition manifests in the dynamics of a many-body system subject to a sudden quench. Focusing on the Lipkin-Meshkov-Glick model initialized in the ground state of the ferromagnetic phase, we demonstrate that the work probability distribution displays non-Gaussian behavior for quenches in the vicinity of the excited state critical point. Furthermore, we show that the entropy of the diagonal ensemble is highly susceptible to critical regions, making it a robust and practical indicator of the associated spectral characteristics. We assess the role that symmetry breaking has on the ensuing dynamics, highlighting that its effect is only present for quenches beyond the critical point. Finally, we show that similar features persist when the system is initialized in an excited state and briefly explore the behavior for initial states in the paramagnetic phase.